He's voiced by Seth Green though, which is kind of fun
1- Captain America: The Winter Soldier
2- Avengers // Guardians of the Galaxy (tie)
4- Iron Man
5- Thor: The Dark World
7- Captain America: The First Avenger
8- Iron Man 2
9- Incredible Hulk
10- Iron Man 3 (I still liked it, but not as much as the rest)
If we're also looking at non-Marvel Studios properties, then X-Men, X2: X-Men United, X-Men: First Class, and X-Men: Days of Future Past all collectively sit near the top, while X-Men 3: The Last Stand, X-Men Origins: Wolverine, and The Wolverine sit lower, near #9. The Fantastic Four and Ghost Rider movies sit well at the bottom. Daredevil, Punisher, and the Blade movies near the middle (Blade 1 a bit higher though; that was fun). Spider-Man 1 and 2, and Amazing Spider-Man 1 and 2 around the #4ish position, and Spider-Man 3 at the very bottom. I haven't seen Elektra or Punisher: War Zone.
"I must not fear. Fear is the mind-killer. Fear is the little-death that brings total obliteration. I will face my fear. I will permit it to pass over me and through me. And when it has gone past I will turn the inner eye to see its path. Where the fear has gone there will be nothing. Only I will remain."
-Bene Gesserit Litany Against Fear